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Lines represent the calculated rate-weighted adsorbate temperatures T ads RW see text. Note the scaling factor of 0. So far, no information is gd-ru001 on the energy transfer during reaction into gd-ru001 i.

One might expect that due to the location of the barrier along the vibrational coordinate, excitation of the interatomic distance d will facilitate the CO associative desorption more than it does excitation of the distance coordinate z between the C—O and the Gd-ru001 surface. These findings imply strong vibrational quenching cooling in reactive trajectories passing the barrier and consequently were taken as indirect evidence for strong nonadiabatic coupling in the N 2 desorption gd-ru001.

However, gd-ru001 has to keep in mind that this vibrational damping of the nascent N 2 molecule relates to locations on the ground state PES beyond the transition state, whereas the gd-ru001 coupling in the excitation step of the fs-laser induced CO association corresponds to the ascending side of the desorption barrier. As a consequence, the nascent CO molecule might be trapped and at least partially thermalized or scattered at this chemisorption well losing memory of the initial activation step. Taborelli, R.

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Allenspach, G. Boffa and M.

Landolt, Phys. Letters 56 gd-ru001 Wissmann Elsevier, Amsterdam, p. Niemantsverdriet, K. Markert, P. Dolle and K.

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